论文标题

超低粘性碰撞:理论和实验状态

Ultracold Sticky Collisions: Theoretical and Experimental Status

论文作者

Bause, Roman, Christianen, Arthur, Schindewolf, Andreas, Bloch, Immanuel, Luo, Xin-Yu

论文摘要

碰撞复合物在分子碰撞中形成为中间状态,通常是短暂的,并且在皮秒内腐烂。然而,在涉及双重分子的超低碰撞中,复合物可以用于毫秒,从而完全改变了碰撞动力学。这可能导致在非反应分子样品中意外的两体丧失。在过去的十年中,这种“粘性”山脉在制备密集和稳定的分子样品的制备方面是一个主要的障碍,尤其是在量子定位方案中。目前,尚未完全理解复合体的行为。例如,在某些情况下,它们的寿命已被衡量的数量级比最近的模型更长。这本身就是一个有趣的问题,而且实际上是相关的问题,因为了解分子复合物可能有助于减轻其有害影响。在这里,我们回顾了该领域最近的实验和理论进步。我们处理分子 - 分子和分子原子碰撞的情况。

Collisional complexes, which are formed as intermediate states in molecular collisions, are typically short-lived and decay within picoseconds. However, in ultracold collisions involving bialkali molecules, complexes can live for milliseconds, completely changing the collision dynamics. This can lead to unexpected two-body loss in samples of nonreactive molecules. During the last decade, such "sticky" collisons have been a major hindrance in the preparation of dense and stable molecular samples, especially in the quantum-degenerate regime. Currently, the behavior of the complexes is not fully understood. For example, in some cases their lifetime has been measured to be many orders of magnitude longer than recent models predict. This is not only an intriguing problem in itself but also practically relevant, since understanding molecular complexes may help to mitigate their detrimental effects. Here, we review the recent experimental and theoretical progress in this field. We treat the case of molecule-molecule as well as molecule-atom collisions.

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