论文标题

对跨金属到建筑物的转变进行巡回量身定位的转移,v $ _2 $ o $ _3 $

Imaging the itinerant-to-localized transmutation of electrons across the metal-to-insulator transition in V$_2$O$_3$

论文作者

Thees, Maximilian, Lee, Min-Han, Bouwmeester, Rosa Luca, Rezende-Gonçalves, Pedro H., David, Emma, Zimmers, Alexandre, Frantzeskakis, Emmanouil, Vargas, Nicolas M., Kalcheim, Yoav, Fèvre, Patrick Le, Horiba, Koji, Kumigashira, Hiroshi, Biermann, Silke, Trastoy, Juan, Rozenberg, Marcelo J., Schuller, Ivan K., Santander-Syro, Andrés F.

论文摘要

在固体中,电子之间的强烈排斥可以抑制其运动,并导致“莫特”金属对绝缘体转变(MIT),这是一种基本现象,其理解一直是超过50年的挑战。一个关键问题是,由于相互作用的增加,波浪状巡回电子如何变为局部状态。但是,从系统的能量和动量分辨的电子结构来观察MIT,这是探测行程和局部状态的唯一直接方法,这是难以捉摸的。 Here we show, using angle-resolved photoemission spectroscopy (ARPES), that in V$_2$O$_3$ the temperature-induced MIT is characterized by the progressive disappearance of its itinerant conduction band, without any change in its energy-momentum dispersion, and the simultaneous shift to larger binding energies of a quasi-localized state initially located near the Fermi level.

In solids, strong repulsion between electrons can inhibit their movement and result in a "Mott" metal-to-insulator transition (MIT), a fundamental phenomenon whose understanding has remained a challenge for over 50 years. A key issue is how the wave-like itinerant electrons change into a localized-like state due to increased interactions. However, observing the MIT in terms of the energy- and momentum-resolved electronic structure of the system, the only direct way to probe both itinerant and localized states, has been elusive. Here we show, using angle-resolved photoemission spectroscopy (ARPES), that in V$_2$O$_3$ the temperature-induced MIT is characterized by the progressive disappearance of its itinerant conduction band, without any change in its energy-momentum dispersion, and the simultaneous shift to larger binding energies of a quasi-localized state initially located near the Fermi level.

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