论文标题

顶点占主导地位的超导性。

Vertex dominated superconductivity in intercalated FeSe

论文作者

Acharya, Swagata, Katsnelson, Mikhail I., van Schilfgaarde, Mark

论文摘要

散装的FESE变得超过9 \,K以下,但是当与碱性元素插入时,临界温度(T $ _ {C} $)几乎被普遍增强了$ \ sim $ 4-5。插入方式如何从原位X射线和中子散射技术中知道结构,但是为什么t $ _ {c} $变化如此之大。在这里,我们表明,即使核自旋松弛率$ {1}/{(t_ {1} t)$,在某些$ \ bf q $ vectors的磁性不稳定性和超导配对顶点之间的增强之间也存在一对一的对应关系。插入修改了平面和层之间的电子筛选。我们定量地删除了超导配对顶点如何从每种此类电子筛选中的变化中获取。插入的FESE提供了超导性的原型示例,其中源自单粒子电子结构的信息似乎不足以说明超导性的起源,即使计算出包括相关效应的信息。我们表明,Intercalation t $ _ {C} $中的五倍增强功能对D $ _ {xy} $的确切位置不敏感,只要$γ$点即可保持接近e $ _ {f} $。最后,我们表明插入还显着软化了集体电荷激发,这表明电子 - phonon相互作用可能在互动的FESE中起作用。

Bulk FeSe becomes superconducting below 9\,K, but the critical temperature (T$_{c}$) is enhanced almost universally by a factor of $\sim$4-5 when it is intercalated with alkali elements. How intercalation modifies the structure is known from in-situ X-ray and neutron scattering techniques, but why T$_{c}$ changes so dramatically is not known. Here we show that there is one-to-one correspondence between the enhancement in magnetic instabilities at certain $\bf q$ vectors and superconducting pairing vertex, even while the nuclear spin relaxation rate ${1}/{(T_{1}T)}$ may not reflect this enhancement. Intercalation modifies electronic screening both in the plane and also between layers. We disentangle quantitatively how superconducting pairing vertex gains from each such changes in electronic screening. Intercalated FeSe provides an archetypal example of superconductivity where information derived from the single-particle electronic structure appears to be insufficient to account for the origins of superconductivity, even when they are computed including correlation effects. We show that the five-fold enhancement in T$_{c}$ on intercalation is not sensitive to the exact position of the d$_{xy}$ at $Γ$ point, as long as it stays close to E$_{F}$. Finally we show that intercalation also significantly softens the collective charge excitations, suggesting the electron-phonon interaction could play some role in intercalated FeSe.

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