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We analyze the energy dependence of the X-ray pulse profile and the phase-resolved spectra (PRS) of the Crab pulsar using observations from the Neutron star Interior Composition Explorer (NICER) and the Hard X-ray Modulation Telescope (Insight-HXMT). We parameterize the pulse profiles and quantify the evolution of these parameters in the broad energy band of 0.4-250 keV. A log-parabola function is used to fit the PRS in 2-250 keV, and the curvature of the spectrum, i.e., the evolution of the photon index with energy, as represented by the parameter \{beta} of the log-parabola model, also changes with phase. The relation of \{beta} and phase has two turning points slightly later than those of the pulse intensity profile, where the values of \{beta} are the lowest, suggesting that the energy-loss rate of the particles is the lowest in the corresponding regions. A three-segment broken-power-law model is also used to fit those PRS. The differences between the hard spectral index and the soft ones have a distribution similar to that of \{beta}, confirming the fitting results of the log-parabola model, while the broken energies are generally higher in the region bridging the two pulses. We find anticorrelations between the spectral indices and the curvature of the log-parabola model fitting and a similar anticorrelation between the spectral indices and broken energies of the broken-power-law model fitting, suggesting a scenario where the highest-energy particles are produced in regions where radiation energy loss is strongest.