论文标题

两个原子的配对相关性和光学镊子中的光相关动力学

Pair Correlations and Photoassociation Dynamics of Two Atoms in an Optical Tweezer

论文作者

Weyland, M., Szigeti, S. S., Hobbs, R. A. B., Ruksasakchai, P., Sanchez, L., Andersen, M. F.

论文摘要

我们在光学镊子中研究了两个激光冷却的$^{85} $ rb原子的光相关动力学,并在许多原子集合中揭示了与光缔合的根本不同的行为。我们在两种原子实验中观察到非指数衰减,该实验无法用单个速率系数描述,并在系统对的相关性中找到其起源。这与许多原子光相关动力学形成鲜明对比,后者由单个速率系数的指数衰减控制。我们还研究了三原子系统中的光相结合,从而探测了从两种原子动力学到多原子动力学的过渡。我们的实验揭示了仅通过控制单个原子才能访问的其他反应动力学,并建议光相关可以测量几个原子系统中的对相关性。它进一步展示了我们对单个原子和分子的量子状态的完全控制,从许多原子实验中提供了无法获得的信息。

We investigate the photoassociation dynamics of exactly two laser-cooled $^{85}$Rb atoms in an optical tweezer and reveal fundamentally different behavior to photoassociation in many-atom ensembles. We observe non-exponential decay in our two-atom experiment that cannot be described by a single rate coefficient and find its origin in our system's pair correlation. This is in stark contrast to many-atom photoassociation dynamics, which are governed by exponential decay with a single rate coefficient. We also investigate photoassociation in a three-atom system, thereby probing the transition from two-atom dynamics to many-atom dynamics. Our experiments reveal additional reaction dynamics that are only accessible through the control of single atoms and suggest photoassociation could measure pair correlations in few-atom systems. It further showcases our complete control over the quantum state of individual atoms and molecules, which provides information unobtainable from many-atom experiments.

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