论文标题
表征离子辐射的FECR:硬度,热扩散性和晶格应变
Characterising Ion-Irradiated FeCr: Hardness, Thermal Diffusivity and Lattice Strain
论文作者
论文摘要
离子辐射的FECR合金可用于理解和预测未来核反应堆结构钢中的中子损伤。先前的研究主要集中在辐射引起的缺陷的结构上,该缺陷通过透射电子显微镜(TEM)探测,以及机械性能的变化。在这些研究中,对具有不同处理历史的样品进行了广泛的辐射条件,这使对缺陷结构和材料特性之间关系的分析变得复杂。此外,很少探索关键特性,例如辐射诱导的热传输和晶格菌株的变化。 在这里,我们提出了一项针对FE3CR,FE5CR和FE10CR二进制合金的系统研究,该合金在室温下植入了20 MeV Fe $^{3+} $离子为0.01 DPA和0.1 dpa的名义剂量。使用纳米指标,瞬态光栅光谱(TGS)和X射线微束LAUE衍射来研究材料中硬度,热扩散率和应变的变化,这是损伤和CR含量的函数。我们的结果表明,CR导致辐射引起的缺陷的保留增加,从而导致硬度和晶格菌株的实质变化。但是,随着损害的增加,热扩散率几乎没有变化,而随着材料中CR含量的增加而显着降解。即使在暴露于名义位移损伤为0.01 DPA的样品中,我们也发现了明显的晶格菌株。晶格应变测量结果预测的缺陷密度明显高于先前研究中观察到的缺陷密度,这表明TEM可能无法完全捕获辐射诱导的缺陷群体。
Ion-irradiated FeCr alloys are useful for understanding and predicting neutron-damage in the structural steels of future nuclear reactors. Previous studies have largely focused on the structure of irradiation-induced defects, probed by transmission electron microscopy (TEM), as well as changes in mechanical properties. Across these studies, a wide range of irradiation conditions has been employed on samples with different processing histories, which complicates the analysis of the relationship between defect structures and material properties. Furthermore, key properties, such as irradiation-induced changes in thermal transport and lattice strain, are little explored. Here we present a systematic study of Fe3Cr, Fe5Cr and Fe10Cr binary alloys implanted with 20 MeV Fe$^{3+}$ ions to nominal doses of 0.01 dpa and 0.1 dpa at room temperature. Nanoindentation, transient grating spectroscopy (TGS) and X-ray micro-beam Laue diffraction were used to study the changes in hardness, thermal diffusivity and strain in the material as a function of damage and Cr content. Our results suggest that Cr leads to an increased retention of irradiation-induced defects, causing substantial changes in hardness and lattice strain. However, thermal diffusivity varies little with increasing damage and instead degrades significantly with increasing Cr content in the material. We find significant lattice strains even in samples exposed to a nominal displacement damage of 0.01 dpa. The defect density predicted from the lattice strain measurements is significantly higher than that observed in previous TEM studies, suggesting that TEM may not fully capture the irradiation-induced defect population.