论文标题

升级IAEA的推荐数据,用于生产PET和SPECT同位素的核反应

Upgrade of IAEA recommended data of selected nuclear reactions for production of PET and SPECT isotopes

论文作者

Hermanne, A., Tárkányi, F. T., Ignatyuk, A. V., Takács, S., Capote, R.

论文摘要

IAEA研究项目专门用于$^{11} $ c,$^{13} $ n,$^{15} $ n,$^{15} $,$^{18} $ f,$^{18} $ f,$^{18} $ f,$^{64} $ cu,and $^cution and positrron和Positiation,在Spect Imaging中使用的两个Gamma发射器的加速器生产,$^{81} $ rb和$^{123} $ i。评估了可用于放射性核素加速器产生的19个带电粒子诱导的反应的横截面,包括不确定性。从Padé拟合到选定和校正的实验数据中获得了所得参考横截面数据,随后推导了积分厚的目标产率。通过PADé最小二乘法估算了拟合结果中的不确定性,并在估计的实验不确定性中添加了4 \%评估的系统不确定性。还将实验数据与卷食文库可用的理论预测进行了比较。 All of the numerical reference cross-section data with their corresponding uncertainties and deduced integral thick target yields are available on-line at the IAEA-NDS medical portal https://www-nds.iaea.org/medportal/ and also at the IAEA-NDS web page https://www-nds.iaea.org/medical/.

An IAEA research project was dedicated to the compilation, evaluation and recommendation of cross-section data for the accelerator production of $^{11}$C, $^{13}$N, $^{15}$O, $^{18}$F, $^{64}$Cu, and $^{124}$I positron-emitting radionuclides clinically used for PET imaging, and for the accelerator production of two gamma emitters, $^{81}$Rb and $^{123}$I, used in SPECT imaging. Cross sections for 19 charged-particle induced reactions that can be employed for radionuclide accelerator production were evaluated including uncertainties. The resulting reference cross-section data were obtained from Padé fits to selected and corrected experimental data, and integral thick target yields were subsequently deduced. Uncertainties in the fitted results were estimated via a Padé least-squares method with the addition of a 4\% assessed systematic uncertainty to the estimated experimental uncertainty. Experimental data were also compared with theoretical predictions available from the TENDL library. All of the numerical reference cross-section data with their corresponding uncertainties and deduced integral thick target yields are available on-line at the IAEA-NDS medical portal https://www-nds.iaea.org/medportal/ and also at the IAEA-NDS web page https://www-nds.iaea.org/medical/.

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