论文标题
在强激光驱动器下的激发能量转移
Excitation Energy Transfer under Strong Laser Drive
论文作者
论文摘要
强分子 - 光相互作用可以控制分子结构和动力学过程。提出了一个具有强激光驱动的模型，以极大地增强共振能传递的分子间距离，其中分子由光腔强烈驱动。观察到能量转移的最佳狂犬病频率和量子产率，这是由于偶极 - 偶极相互作用和分子腔耦合之间的权衡。当应用某些RABI频率下的强驱动器时，与我们的模型中观察到了较大的有效能量传递范围和距离较慢的衰减速率，距离距离较慢。我们的工作阐明了分子极化子中合作能量转移的光谱研究。
Strong molecule-light interaction enables the control of molecular structures and dynamical processes. A model with strong laser drive is proposed to greatly enhance the intermolecular distance of resonant energy transfer, where the molecules are strongly driven by an optical cavity. The optimal Rabi frequency and quantum yield of energy transfer are observed, resulting from the trade off between dipole-dipole interaction and molecule-cavity coupling. When the strong drive at certain Rabi frequency is applied, a larger spatial range of effective energy transfer and a slower decay rate with the distance compared to the Förster mechanism of resonant energy transfer are observed in our model. Our work sheds light on spectroscopic study of the cooperative energy transfer in molecular polaritons.
