论文标题

金属Perovskites gdrh $ _3 $ c $ _ {1-x} $ b $ _x $的不稳定性和磁基状态的演变

Instability and evolution of the magnetic ground state in metallic perovskites GdRh$_3$C$_{1-x}$B$_x$

论文作者

Pandey, Abhishek, Singh, A. K., Dan, Shovan, Ghosh, K., Das, I., Tripathi, S., Kumar, U., Ranganathan, R., Johnston, D. C., Mazumdar, Chandan

论文摘要

我们报告了金属钙钛矿GDRH $ _3 $ c $ _ {1-x} $ b $ _x $($ 0.00 \ le x \ le x \ le 1.00 $)的五个组成的结构,磁,电气传输和热性能的调查。我们的结果表明,所有这五个组合物在低温下都经过磁性秩序,但是在碳和富含硼的组合物中,有序状态的性质有显着差异,其中前者显示了振幅调节的磁性结构的特征,后者表现出相等的抗强度抗抗激素的证据。我们还观察到在构图无序化合物中传导载​​体极化的明显磁场依赖性演变。结果表明,该系统在磁不稳定性的距离上位于磁不稳定性的附近,其中控制参数中的较小变化(例如晶格常数和/或电子密度)导致基态不同。

We report investigations of the structural, magnetic, electrical transport and thermal properties of five compositions of the metallic perovskite GdRh$_3$C$_{1-x}$B$_x$ ($0.00 \le x \le 1.00$). Our results show that all the five compositions undergo magnetic ordering at low temperatures, but the nature of the ordered state is significantly different in the carbon- and the boron-rich compositions, where the former shows signatures of an amplitude-modulated magnetic structure and the latter exhibits evidences of an equal-moment incommensurate antiferromagnetic ordering. We also observe a remarkable field-dependent evolution of conduction carrier polarization in the compositionally disordered compounds. The outcomes indicate that this system is energetically situated in proximity to a magnetic instability where small variations in the control parameter(s), such as lattice constant and/or electron density, lead to considerably different ground states.

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