论文标题

激子相互作用引起的旋转分裂$ _2 $单层

Exciton interaction induced spin splitting in MoS$_2$ monolayer

论文作者

Li, Yao, Li, G., Zhai, Xiaokun, Xiong, Shi Fu, Liu, Hongjun, Wang, Xiao, Chen, Haitao, Gao, Ying, Zhang, Xiu, Liu, Tong, Ren, Yuan, Ma, Xuekai, Fu, Hongbin, Gao, T.

论文摘要

通过在循环极化的CW激光器下以$ 13 $ K的价格泵送Mos $ _2 $单层,我们观察到激子的能量红移,这破坏了与旋转相反旋转的B激子之间的退化。能量分裂会随着激光功率达到多达$ 18 $ MEV的单调增加,而温度会降低。理论上可以通过同时考虑带段的带隙重生化来解释这种现象,从而产生了红移和激子 - 外激体库仑交换相互作用,该相互作用负责旋转依赖性分裂。我们的结果提供了一个简单的方案,可以控制Mos $ _2 $单层中的山谷自由度,并提供了一种可访问的方法,用于调查此类材料中多体激子激子相互作用。

By pumping nonresonantly a MoS$_2$ monolayer at $13$ K under a circularly polarized cw laser, we observe exciton energy redshifts that break the degeneracy between B excitons with opposite spin. The energy splitting increases monotonically with the laser power reaching as much as $18$ meV, while it diminishes with the temperature. The phenomenon can be explained theoretically by considering simultaneously the bandgap renormalization which gives rise to the redshift and exciton-exciton Coulomb exchange interaction which is responsible for the spin-dependent splitting. Our results offer a simple scheme to control the valley degree of freedom in MoS$_2$ monolayer and provide an accessible method in investigating many-body exciton exciton interaction in such materials.

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